{"id":12195,"date":"2020-07-30T00:00:20","date_gmt":"2020-07-29T16:00:20","guid":{"rendered":"https:\/\/www.science.nus.edu.sg\/?p=12195"},"modified":"2020-07-30T10:39:37","modified_gmt":"2020-07-30T02:39:37","slug":"incorporating-ferromagnetism-and-superconductivity-together-in-a-single-layer-of-molecular-superlattice","status":"publish","type":"post","link":"https:\/\/www.science.nus.edu.sg\/blog\/2020\/07\/incorporating-ferromagnetism-and-superconductivity-together-in-a-single-layer-of-molecular-superlattice\/","title":{"rendered":"Incorporating ferromagnetism and superconductivity together in a single layer of molecular superlattice"},"content":{"rendered":"<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">NUS scientists have demonstrated an interlayer-space confined chemical design (ICCD) method for the synthesis of single-atom doped <\/span><span lang=\"EN-US\">tantalum disulfide (<\/span><span lang=\"EN-GB\">TaS<sub>2<\/sub>) molecular superlattice, where ferromagnetism was successfully introduced in the superconducting TaS<sub>2<\/sub> layers.<\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-US\">The interplay between superconductivity and ferromagnetism creates numerous exotic physical phenomena, which can be harnessed for next generation device applications. The integration of these two competing phases is usually achieved by vertically stacking superconductor and ferromagnetic layers one after another. \u00a0Controllable synthesis of hybrid atomic layers which accommodate both superconductivity and ferromagnetism remain a considerable challenge<\/span><span lang=\"EN-US\">. <\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">A research team led by Prof LU Jiong from the Department of Chemistry, NUS has demonstrated that the incorporation of isolated cobalt (Co) atoms into superconducting TaS<sub>2<\/sub> layers can induce local magnetic moments and ferromagnetic coupling. This creates a material with ferromagnetic and superconducting domains within <\/span><span lang=\"EN-GB\">a single atomic layer. In comparison with <\/span><span lang=\"EN-US\">conventional vertically stacked structures, integrating these two competing phases into a single layer not only offers improved flexibility in device design and fabrication, it also opens up new potential applications. <\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">Prof Lu\u2019s team developed this new approach, called ICCD,<\/span><span lang=\"EN-GB\"> <\/span><span lang=\"EN-GB\">for the simultaneous intercalation and chemical modification of bulk 2H-TaS<sub>2<\/sub>, where ferromagnetism is introduced into the TaS<sub>2<\/sub> material while retaining its superconductivity properties (Figure A). Inserting tetrabutylammonium molecules into the space between layers of TaS<sub>2<\/sub> opens up the spacing between them and allows Co<sup>2+<\/sup> ions to be integrated into the structure. The researchers found that the Co<sup>2+<\/sup> ions either replaced the tantalum (Ta) atom or got adsorbed at a hollow site (between two Ta atoms) (Figure B). This ICCD strategy can potentially be applied to various metal ions, enabling a versatile and scalable synthesis of a class of molecular superlattices with tailored properties via interlayer modification.<\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">The team\u2019s experimental results, together with theoretical calculations carried out by Prof <\/span><span lang=\"EN-GB\">Yuanping FENG\u2019s <\/span><span lang=\"EN-GB\">group from<\/span><span lang=\"EN-GB\"> <\/span><span lang=\"EN-US\">the <\/span><span lang=\"EN-GB\">Department of Physics, NUS show that the orbital-selected <i>p<\/i>&#8211;<i>d<\/i> hybridisation between Co and their neighbouring Ta and S atoms induces local magnetic moments and ferromagnetic coupling (Figure C), presumably mediated through a mechanism known as the Ruderman-Kittel-Kasuya-Yosida exchange interaction.<\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">Prof Lu said, &#8220;We envisage that our findings <\/span><span lang=\"EN-GB\">of<\/span><span lang=\"EN-GB\"> the interlayer-space confined chemical design will provide a new chemical route to engineer artificial molecular superlattice of layered materials with exotic and antagonistic properties for desired functionalities.\u201d<\/span><\/span><\/p>\n<p><img fetchpriority=\"high\" decoding=\"async\" src=\"https:\/\/www.science.nus.edu.sg\/wp-content\/uploads\/2020\/07\/236._Lu_Jiong_CHM_1.jpg\" alt=\"\" class=\"alignnone  wp-image-12198\" width=\"646\" height=\"382\" srcset=\"https:\/\/www.science.nus.edu.sg\/wp-content\/uploads\/2020\/07\/236._Lu_Jiong_CHM_1.jpg 850w, https:\/\/www.science.nus.edu.sg\/wp-content\/uploads\/2020\/07\/236._Lu_Jiong_CHM_1-300x178.jpg 300w, https:\/\/www.science.nus.edu.sg\/wp-content\/uploads\/2020\/07\/236._Lu_Jiong_CHM_1-768x454.jpg 768w\" sizes=\"(max-width: 646px) 100vw, 646px\" \/><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\">Figure (A) provides a schematic illustration of<\/span><span lang=\"EN-GB\"> the interlayer-space confined chemical design (ICCD) method for the synthesis of tantalum disulfide (TaS<sub>2<\/sub>) molecular superlattice with the superconducting regions and ferromagnetic regions in a single atomic layer<\/span><span lang=\"EN-GB\">. Figure (B) includes the high-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) images showing the substituted Co atom (Co<sub>Ta<\/sub>) and hollow-site Co atom (Co<sub>HS<\/sub>) within the TaS<sub>2<\/sub> material. Figure (C) is the spin density plots of the TaS<sub>2<\/sub> monolayer with Co<sub>Ta<\/sub> (left) and Co<sub>HS<\/sub> (right) showing the introduction of ferromagnetism into the TaS<sub>2<\/sub> material. \u00a0<\/span><span lang=\"EN-GB\">[Credit: Advanced Materials]<\/span><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\"><span lang=\"EN-GB\"><\/span><b><span lang=\"EN-GB\">Reference<\/span><\/b><\/span><\/p>\n<p><span style=\"font-family: arial, helvetica, sans-serif; font-size: 12pt;\" lang=\"EN-GB\">Li Z; Zhang X; Zhao X; Li J; Herng T; Xu H; Lin F; Lyu P; Peng X; Yu W; Hai X; Chen C; Yang H; Martin J; Lu J; Luo X; Neto A.; Pennycook S; Ding J; Feng Y; Lu J* \u201cImprinting ferromagnetism and superconductivity in single atomic layers of molecular superlattices\u201d ADVANCED MATERIALS DOI: 10.1002\/adma.201907645 Published: 2020.<\/span><\/p>\n","protected":false},"excerpt":{"rendered":"<p>NUS scientists have demonstrated an interlayer-space confined chemical design (ICCD) method for the synthesis of single-atom doped tantalum disulfide (TaS<sub>2<\/sub>) &#8230;<\/p>\n","protected":false},"author":16,"featured_media":12197,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"_acf_changed":false,"footnotes":""},"categories":[23,13],"tags":[],"class_list":["post-12195","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-advanced-materials","category-research-news"],"acf":[],"yoast_head":"<!-- This site is optimized with the Yoast SEO Premium plugin v23.6 (Yoast SEO v23.6) - https:\/\/yoast.com\/wordpress\/plugins\/seo\/ -->\n<title>Incorporating ferromagnetism and superconductivity together in a single layer of molecular superlattice - NUS Faculty of Science<\/title>\n<meta name=\"robots\" content=\"index, follow, max-snippet:-1, max-image-preview:large, max-video-preview:-1\" \/>\n<link rel=\"canonical\" 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